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CRYSTALLIZATION BEHAVIOR continued


Figure 2 – Crystallization exotherms for cap samples.


Figure 1 – Example of Avrami analysis using linear form from X(t) = 0.2 to X(t) = 0.8.


Experimental Samples Samples used were marker pen caps in various colors purchased from a


local office supplier. (They are polypropylene but the author does not have access to the formulation; the base resin is likely the same formulation.) Sample colors include black, red, yellow, brown, orange, green, blue and purple. A cap made from polypropylene containing no pigments was used as a reference.


Instrument and experimental parameters 1. Instrument: Discovery DSC 2500 (TA Instruments, New Castle, Del.)


2. Sample mass: 5 mg nominal 3. Purge gas: N2


at 50 mL/min


Table 2 – Summary of single-point Avrami analysis Sample Red


TC


Brown Black


Purple Blue


Orange Green Yellow


No colorant °C


122.7 113.9 124.2 130.8 129.4 122.8 127.0 121.9 110.7


n


2.053 2.956 2.786 1.896 2.472 2.103 2.271 2.287 3.094


Figure 3 – Crystallized fraction as a function of temperature.


k


2.507 3.071 6.088 3.282 6.515 5.421 6.299 6.992 1.200


t1/2


(min)


0.535 0.604 0.458 0.440 0.404 0.376 0.378 0.364 0.837


τ (reciprocal half-time-min-1 1.87


1.66 2.18 2.27 2.48 2.66 2.65 2.75 1.19


)


AMERICAN LABORATORY


12


JANUARY/FEBRUARY 2017


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